122 research outputs found
Chiral Perturbation Theory tests at NA48 and NA62-RK experiments at CERN
Final results from an analysis of about 400 K ± → π ± γγ rare decay candidates collected by the NA48/2 and NA62-RK experiments at CERN during low intensity runs with minimum
bias trigger configurations are presented. The results include a model-independent decay rate measurement and fits to Chiral Perturbation Theory (ChPT) description. The data
support the ChPT prediction for a cusp in the di-photon invariant mass spectrum at the two pion threshold
Search for the dark photon in decays
A sample of fully reconstructed
decay candidates collected by the NA48/2 experiment at CERN in 2003--2004 is
analysed to search for the dark photon () production in the decay followed by the prompt decay. No signal is observed,
and an exclusion region in the plane of the dark photon mass and
mixing parameter is established. The obtained upper limits on
are more stringent than the previous limits in the mass range
9~
m MeV/c^2<70~
m MeV/c^2. The NA48/2 sensitivity to the dark
photon production in the decay is also evaluated
Ultrafast adsorbate excitation probed with sub-ps resolution XAS
We use a pump-probe scheme to measure the time evolution of the C K-edge
X-ray absorption spectrum (XAS) from CO/Ru(0001) after excitation by an
ultrashort high-intensity optical laser pulse. Due to the short duration of the
X-ray probe pulse and precise control of the pulse delay, the
excitation-induced dynamics during the first ps after the pump can be resolved
with unprecedented time resolution. By comparing with theoretical (DFT)
spectrum calculations we find high excitation of the internal stretch and
frustrated rotation modes occurring within 200 fs of laser excitation, as well
as thermalization of the system in the ps regime. The ~100 fs initial
excitation of these CO vibrational modes is not readily rationalized by
traditional theories of nonadiabatic coupling of adsorbates to metal surfaces,
e. g. electronic frictions based on first order electron-phonon coupling or
transient population of adsorbate resonances. We suggest that coupling of the
adsorbate to non-thermalized electron-hole pairs is responsible for the
ultrafast initial excitation of the modes.Comment: 16 pages, 16 figures. To be published in Physical Review Letters:
https://journals.aps.org/prl/accepted/c1070Y74M8b18063d9cd0221b000631d50ef7a24
Ultrafast Adsorbate Excitation Probed with Subpicosecond-Resolution X-Ray Absorption Spectroscopy
We use a pump-probe scheme to measure the time evolution of the C K-edge x-ray absorption spectrum from CO/Ru(0001) after excitation by an ultrashort high-intensity optical laser pulse. Because of the short duration of the x-ray probe pulse and precise control of the pulse delay, the excitation-induced dynamics during the first picosecond after the pump can be resolved with unprecedented time resolution. By comparing with density functional theory spectrum calculations, we find high excitation of the internal stretch and frustrated rotation modes occurring within 200 fs of laser excitation, as well as thermalization of the system in the picosecond regime. The ∼100 fs initial excitation of these CO vibrational modes is not readily rationalized by traditional theories of nonadiabatic coupling of adsorbates to metal surfaces, e.g., electronic frictions based on first order electron-phonon coupling or transient population of adsorbate resonances. We suggest that coupling of the adsorbate to nonthermalized electron-hole pairs is responsible for the ultrafast initial excitation of the modes
Atom-Specific Probing of Electron Dynamics in an Atomic Adsorbate by Time-Resolved X-Ray Spectroscopy
The electronic excitation occurring on adsorbates at ultrafast timescales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of x-ray absorption spectroscopy (XAS) and x-ray emission spectroscopy (XES) of a simple well-known adsorbate prototype system, namely carbon (C) atoms adsorbed on a nickel [Ni(100)] surface, following intense laser optical pumping at 400 nm. We observe ultrafast (∼100 fs) changes in both XAS and XES showing clear signatures of the formation of a hot electron-hole pair distribution on the adsorbate. This is followed by slower changes on a few picoseconds timescale, shown to be consistent with thermalization of the complete C/Ni system. Density functional theory spectrum simulations support this interpretation
Atom-Specific Probing of Electron Dynamics in an Atomic Adsorbate by Time-Resolved X-ray Spectroscopy
The electronic excitation occurring on adsorbates at ultrafast time scales
from optical lasers that initiate surface chemical reactions is still an open
question. Here, we report the ultrafast temporal evolution of X-ray absorption
spectroscopy (XAS) and X-ray emission spectroscopy (XES) of a simple well known
adsorbate prototype system, namely carbon (C) atoms adsorbed on a nickel
(Ni(100)) surface, following intense laser optical pumping at 400 nm. We
observe ultrafast (~100 fs) changes in both XAS and XES showing clear
signatures of the formation of a hot electron-hole pair distribution on the
adsorbate. This is followed by slower changes on a few ps time scale, shown to
be consistent with thermalization of the complete C/Ni system. Density
functional theory spectrum simulations support this interpretation.Comment: 33 pages, 12 figures. Submitted to Physical Review Letter
Symmetry-Resolved CO Desorption and Oxidation Dynamics on O/Ru(0001) Probed at the C K-edge by Ultrafast X-Ray Spectroscopy
We report on carbon monoxide desorption and oxidation induced by 400 nm femtosecond laser excitation on the O/Ru(0001) surface probed by time-resolved x-ray absorption spectroscopy (TR-XAS) at the carbon K-edge. The experiments were performed under constant background pressures of CO (6 × 10−8 Torr) and O2 (3 × 10−8 Torr). Under these conditions, we detect two transient CO species with narrow 2π* peaks, suggesting little 2π* interaction with the surface. Based on polarization measurements, we find that these two species have opposing orientations: (1) CO favoring a more perpendicular orientation and (2) CO favoring a more parallel orientation with respect to the surface. We also directly detect gas-phase CO2 using a mass spectrometer and observe weak signatures of bent adsorbed CO2 at slightly higher x-ray energies than the 2π* region. These results are compared to previously reported TR-XAS results at the O K-edge, where the CO background pressure was three times lower (2 × 10−8 Torr) while maintaining the same O2 pressure. At the lower CO pressure, in the CO 2π* region, we observed adsorbed CO and a distribution of OC–O bond lengths close to the CO oxidation transition state, with little indication of gas-like CO. The shift toward “gas-like” CO species may be explained by the higher CO exposure, which blocks O adsorption, decreasing O coverage and increasing CO coverage. These effects decrease the CO desorption barrier through dipole–dipole interaction while simultaneously increasing the CO oxidation barrier
Search for heavy neutral lepton production in K+ decays
A search for heavy neutral lepton production in K + decays using a data sample collected with a minimum
bias trigger by the NA62 experiment at CERN in 2015 is reported. Upper limits at the 10−7 to 10−6 level
are established on the elements of the extended neutrino mixing matrix |Ue4|
2 and |Uμ4|
2 for heavy
neutral lepton mass in the ranges 170–448 MeV/c2 and 250–373 MeV/c2, respectively. This improves on
the previous limits from HNL production searches over the whole mass range considered for |Ue4|2 and
above 300 MeV/c2 for |Uμ4|2
SARS-CoV-2 diagnosis and viral load methods based on quantitative RT-PCR
En diciembre de 2019, se produjo un nuevo brote de enfermedad por coronavirus (COVID-19) en Wuhan, China. El síndrome respiratorio agudo severo-coronavirus-2 (SARS-CoV-2), que es el séptimo coronavirus conocido que infecta a los humanos, es altamente infeccioso y se ha expandido rápidamente en todo el mundo desde su descubrimiento. El diagnóstico de la infección por SARS-CoV-2 se basa en la detección del genoma viral (ARN) a través de técnicas de biología molecular. Con este fin, se extrae el ARN total para su posterior detección mediante PCR cuantitativa en tiempo real (RT-qPCR). Las pruebas cuantitativas de ácidos nucleicos se han convertido en el “estándar de oro” para el diagnóstico y guía en la toma de decisiones clínicas. Sin embargo, los ensayos de RT-qPCR dirigidos al SARS-CoV-2 tienen varios desafíos, especialmente en términos de diseño de cebadores / sondas y de desarrollo de metodologías que permitan estimar la carga viral en pacientes con diagnóstico de COVID-19.In December 2019, a new coronavirus disease (COVID-19) outbreak occurred in Wuhan, China. Severe acute respiratory syndrome-coronavirus-2 (SARS-CoV-2), which is the seventh coronavirus known to infect humans, is highly contagious and has rapidly expanded worldwide since its discovery. Quantitative nucleic acid testing has become the gold standard for diagnosis and guiding clinical decisions regarding the use of antiviral therapy. Total RNA is purified for subsequent SARS-CoV-2 detection by a real time quantitative RT-PCR (RT-qPCR). However, the RT-qPCR assays targeting SARS-CoV-2 have a number of challenges, especially in terms of primer / probe design and in the development of methodologies to estimate viral load in patients diagnosed with COVID-19.Este proyecto ha sido financiado por el Programa de Articulación y Fortalecimiento Federal de las Capacidades en Ciencia y Tecnología COVID-19 del Ministerio de Ciencia, Tecnología e Innovación de Argentina. (Proyecto BUE 21).Secretaría de Ciencia y Técnic
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